Classification of Aggregates Using Multispectral Two-Dimensional Angular Light Scattering Simulations

Molecules. 2022 Oct 8;27(19):6695. doi: 10.3390/molecules27196695.

Abstract

Airborne particulate matter plays an important role in climate change and health impacts, and is generally irregularly shaped and/or forms agglomerates. These particles may be characterized through their light scattering signals. Two-dimensional angular scattering from such particles produce a speckle pattern that is influenced by their morphology (shape and material composition). In what follows, we revisit morphological descriptors obtained from computationally generated light scattering patterns from aggregates of spherical particles. These descriptors are used as inputs to a multivariate statistical algorithm and then classified via supervised machine learning algorithms. The classification results show improved accuracy over previous efforts and demonstrate the utility of the proposed morphological descriptors.

Keywords: T-matrix; aggregates; classification; clusters; light scattering; machine learning.

MeSH terms

  • Algorithms*
  • Particulate Matter*
  • Scattering, Radiation

Substances

  • Particulate Matter